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Valeria D. Kleiman
Assistant Professor
of Chemistry
Department of Chemistry
University of Florida
VOICE: (352) 392-4656
EMAIL: kleiman@chem.ufl.edu
HOMEPAGE: http://www.chem.ufl.edu/~kleiman/
Research Interests
Ultrafast
Spectroscopy
The processes of interest
occur very fast (10-15-10-10sec). These events are triggered by the absorption
of energy from a laser pulse. After excitation, the systems can undergo
several changes, involving redistribution of the energy, lose of coherence,
formation of intermediates, etc. The evolution of those changes provides
useful information to understand the light-matter interactions. Since
the temporal evolutions are extremely fast, it is necessary to probe the
system in time-scales faster that the times it takes them to evolve.
In general, ultrafast
spectroscopy techniques involve an initial step (excitation by a short
laser pulse) followed by the probing of the evolution of an optical transition
(through absorption, scattering or photoluminescence) . To probe the evolution
of a fast process we utilize techniques equivalent to the stroboscopic
method develop by Harold "Doc" Edgerton.
Conjugated
polymers
New materials with novel photophysical properties are crucial for developing
revolutionary molecular-photonic and -electronic components. Over the
past two decades, conjugated polymers have emerged as materials exhibiting
valuable properties in optical sensing, energy transport, and light harvesting.
Understanding the optical properties of these materials depends primarily
on the investigation of energy and charge transfer mechanisms. Our research
is focused on the study of poly-conjugated molecules and their photo-physical
properties. The goal is to understand novel properties arising not from
the accumulation of single units, but those that derive from the macromolecule
as a whole. Central to the project is the use of ultrafast spectroscopy
to study energy transport in conjugated polymers whose electronic and
optical properties can be chemically controlled at the molecular level.
We concentrate our
efforts in the areas of energy transfer and storage, and the search for
non-linear properties that can yield new materials for IR sensors, artificial
antennae, and energy conversion. This objective will be achieved by research
of energy-transport and intra- and inter-chain exciton migration mechanisms
in linear (ionic polymers) and dendrimer-like molecules.

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